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Abstract

Environmental applications of carbon nanotubes (CNTs) have recently attracted worldwide attentiondue to their excellent adsorption capacities and promising physical, chemical and mechanical properties, as well asthe preparation of novel membranes with attractive features for water purification. This paper critically reviews therecent progress on the preparation and applications of CNT based membranes in water and wastewater treatment. Various synthesis techniques for the preparation of CNT based membranes are discussed. The functionalization ofCNTs, which involves chemical/physical modification of pristine CNTs with different types of functional groups,improves the capabilities of CNT for water and wastewater treatment and/or removal of waterborne contaminants.The CNT-based membrane applications are found to possess a variety of advantages, including improving waterpermeability, high selectivity and antifouling capability. However, their applications at full scale are still limitedby their high cost. Finally, we highlight that CNT membranes with promising removal efficiencies for respectivecontaminants can be considered for commercialization and to achieve holistic performance for the purpose ofwater treatment and desalination. This paper may provide an insight for the development of CNT based membranesfor water purification in the future. With their tremendous separation performance, low biofouling potential andultra-high water flux, CNT membranes have the potential to be a leading technology in water treatment, especiallydesalination.
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Authors and Affiliations

Michał Bodzek
1
ORCID: ORCID
Krystyna Konieczny
2
ORCID: ORCID
Anna Kwiecińska-Mydlak
3
ORCID: ORCID

  1. Institute of Environmental Engineering Polish Academy of Sciences, Poland
  2. Silesian University of Technology, Faculty of Energy and Environmental Engineering, Poland
  3. Institute for Chemical Processing of Coal, Poland
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Abstract

Many tons of micro- and nano-sized plastic particles enter the aquatic environment every year, due to increasing plastic production, with the consequent risk of microplastics contaminating our environment. Addressing this multifaceted threat requires innovative technologies that can efficiently remove microplastics from the environment. Therefore, there is an urgent need to study the efficiency of the removal of microplastics by different water and wastewater treatment technologies. After short overviewed the source, occurrence, and potential adverse impacts of microplastics to human health, we then identified promising technologies for microplastics removal, including physical, chemical, and biological approaches. A detailed analysis of the advantages and limitations of different techniques was provided. According to literature data, the performance of microplastics removal is as follows: membrane bioreactor (>99%) > activated sludge process (~98%) > rapid sand filtration (~97.1%) > dissolved air floatation (~95%) > electrocoagulation (>90%) > constructed wetlands (88%). Chemical treatment methods such as coagulation, magnetic separation, Fenton, photo-Fenton and photocatalytic degradation also show moderate to high efficiency of microplastics removal. Hybrid treatment such as the MBR-UF/RO system, coagulation followed by ozonation, adsorption, dissolved air flotation, filtration, and constructed wetlands based hybrid technologies have shown very promising results in the effective removal of microplastics. Lastly, research gaps in this area are identified, and suggestions for future perspectives are provided. We concluded this review with the current challenges and future research priorities, which will guide us through the path addressing microplastics contamination.
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Authors and Affiliations

Michał Bodzek
1
ORCID: ORCID
Alina Pohl
1

  1. Institute of Environmental Engineering Polish Academy of Sciences, Zabrze, Poland

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